Multielectron oxidation in a ferromagnetically coupled dinickel(ii) triple mesocate

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Multielectron oxidation in a ferromagnetically coupled dinickel(ii) triple mesocate.

Triple-stranded dinuclear nickel(ii) complexes of the meso-helicate type have been obtained from the new N,N'-1,3-phenylenebis(pyrazine-2-carboxamidate) ligand; they possess a multielectron redox behaviour featuring up to four stepwise, one-electron oxidation reactions of the two ferromagnetically coupled Ni(II) ions to afford the putative high-valent dinickel(iii) and dinickel(iv) species, as ...

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ژورنال

عنوان ژورنال: Chemical Communications

سال: 2015

ISSN: 1359-7345,1364-548X

DOI: 10.1039/c5cc03544a